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Double-Headed Streamer in Nitrogen
Introduction
Streamers are transient filamentary electric discharges that can develop in a nonconducting background in the presence of an intense electric field. These discharges can attain high electron number density and, consequently, a high concentration of chemical active species that are relevant for numerous applications.
The propagation of streamers is driven by very nonlinear dynamics that involve very steep density gradients and high space-charge density distributed in very thin layers. The charge separation at the front (or head) of the streamer generates intense electric fields that are responsible for sharp ionization fronts propagating into the neutral medium.
In negative (anode directed) streamers, ionizing electrons are accelerated outward by the space-charge (the streamer extends toward the anode). These high energy electrons may have been transported by drift or diffusion, or created by another mechanism that provides pre-ionization ahead of the streamer such as photoionization or ionization from runway electrons. In positive (or cathode directed) streamers the space-charge field in the streamer head accelerates the electrons inward. Consequently, the ionizing electrons must be produced by a pre-ionization mechanism. The pre-ionization of the streamer is a complex subject that is believed to be critical for both negative and positive streamers propagation and is still under investigation. This document is an introduction to streamer modeling with focus on basic concepts of streamer propagation. With that in mind it is followed a simplified approach where all pre-ionization is neglected and only negative streamers are discussed.
This example presents a study of a double-headed streamer. An initial seed of electrons is placed between two electrodes spaced by 1 cm to which a voltage of 52 kV is applied (providing a constant initial electric field of 52 kV/cm). A negative and positive streamers propagate towards the electrodes. The electron density, electric field, and the propagation speed of the streamer agrees well with simulation results from Ref. 1.
Model Definition
The model is two dimensional and describes the transient behavior of an initial electron seed in the presence of a strong electric field using fluid-type equations.
The model solves the electron and ion continuity and momentum equations, in the drift-diffusion approximation, self-consistently coupled with Poisson’s equation. The local field approximation is used, which means that transport and source coefficients are assumed to be well parameterized through the reduced electric field (E/N). In the local field approximation the fluid equation for the mean electron energy is not solved, which reduces significantly the complexity of the numerical problem.
The local field approximation is valid in a situation where the rate of electron energy gain from the electric field is locally balanced by the energy loss rate. When this condition is met the electrons are said to be in local equilibrium with the electric field and the electron mean properties can be expressed as a function the reduced electric field.
Domain Equations
The electron density is computed by solving the drift-diffusion equation for the electron density.
(1)
For more detailed information on electron transport, see the section Theory for the Drift Diffusion Interface in the Plasma Module User’s Guide. The source coefficients in the above equation can be determined by the plasma chemistry using rate coefficients
(2)
where xj is the mole fraction of the target species for reaction j, kj is the rate coefficient for reaction j (SI unit: m3/s), and Nn is the total neutral number density (SI unit: 1/m3). For drift-dominated discharges it is better practice to use Townsend coefficients instead of rate coefficients to define reaction rates Ref. 2. When Townsend coefficients are used, the electron source term is given by:
(3)
where αj is the Townsend coefficient for reaction j (m2) and Γe is the electron flux as defined above (1/(m2·s)). Townsend coefficients can increase the stability of the numerical scheme when the electron flux is field driven as is the case with streamers.
For heavy species, the following equation is solved for the mass fraction of each species:
(4)
For detailed information on the transport of the heavy species, see the section Theory for the Heavy Species Transport Interface in the Plasma Module User’s Guide.
The electrostatic field is computed using Poisson’s equation
(5)
The space charge density ρ is automatically computed based on the plasma chemistry specified in the model using the formula
(6)
For detailed information about electrostatics, see Theory for the Electrostatics Interface in the Plasma Module User’s Guide.
Boundary Conditions
The present simulation is arranged in a way that the charged particle interaction with the surfaces does not influence much the streamer propagation. Nevertheless boundary conditions must be given. For electrons a fixed electron density of 1014 cm-3 is set at the electrodes and the default zero flux boundary condition is set at the right boundary. For ions the default zero flux is applied to all boundaries.
For Poisson’s equation, an electric potential of 0 V and 52 kV is set at the bottom and top electrodes, respectively, and the default zero charge boundary condition is applied at the right boundary.
Plasma Chemistry
The chemistry of a plasma sustained in nitrogen can be very complex and a detailed study of the main excited states could easily have hundreds of reactions. The main goal of this model is to study the charge particle density profiles in the presence of strong electric fields. With this in mind, the model includes a single ionization reaction, as presented in Table 1, that correctly describes the creation of charged species in a background of nitrogen. This work uses the Townsend coefficient as a function of reduced electric field provided in Ref. 1.
Δε (eV)
Results and Discussion
The results in this section are for a double-headed streamer propagating in a background gas kept at a constant density as obtained by the ideal gas law at atmospheric pressure and at a temperature of 293.15 K. There is a general good agreement with the results from the model here presented and the ones from Ref. 1.
Figure 1, Figure 2, and Figure 3 show 2d plots of the electron density, space charge density, and electric potential at 2.5 ns. Figure 4 and Figure 5 present the spatial distribution of the electron and ion densities, and the z component of the electric field for several instants during the streamer simulation.
Starting from the center, two streamers develop toward the electrodes. These streamers have different propagation mechanisms that result in different morphology and propagation speeds. The top streamer is anode directed and develops a negative space-charge density since the electric field pulls electrons ahead of the streamer. The bottom streamer is cathode directed and the electrons are drifting in the opposite direction of the streamer propagation. The propagation of the cathode-directed streamer is only possible because it is given a high enough background electron density. Note how the quasineutral streamer body shields the electric field to very small values causing the electrons to cool down.
Figure 3 and Figure 5 can be compared with figures 6 and 7 of Ref. 1. In general, the agreement is very good with the velocity of propagation and the spread being captured accurately.
Figure 1: Electron number density at 2.5 ns.
Figure 2: Space charge density and electric potential at 2.5 ns.
Figure 3: Contours of the electron number density at 2.5 ns. Compare with figure 6 of Ref. 1.
Figure 4: Spatial distribution along the axis of symmetry of the electron (colored solid lines) and ion number density (black dashed lines) for several time instants during the streamer propagation.
Figure 5: Spatial distribution along the axis of symmetry of the z component of the electric field for several time instants during the streamer propagation. Compare with figure 7 of Ref. 1
References
1. D. Bessieres, J. Paillol, A. Bourdon, P. Segur, and E. Marode, “A new one-dimensional moving mesh method applied to the simulation of streamer discharges,” J. Phys. D: Appl. Phys., vol. 40, pp. 6559–6570, 2007.
2. M.A. Lieberman and A.J. Lichtenberg, Principles of Plasma Discharges and Materials Processing, John Wiley & Sons, 2005.
Application Library path: Plasma_Module/Direct_Current_Discharges/streamer_2d
Modeling Instructions
From the File menu, choose New.
New
In the New window, click  Model Wizard.
Model Wizard
1
In the Model Wizard window, click  2D Axisymmetric.
2
In the Select Physics tree, select Plasma>Plasma (plas).
3
Click Add.
4
Click  Study.
5
In the Select Study tree, select General Studies>Time Dependent.
6
Geometry 1
Create the simulation geometry. Add a layer to define a region where the mesh is going to be refined.
1
In the Model Builder window, under Component 1 (comp1) click Geometry 1.
2
In the Settings window for Geometry, locate the Units section.
3
From the Length unit list, choose cm.
Rectangle 1 (r1)
1
In the Geometry toolbar, click  Rectangle.
2
In the Settings window for Rectangle, click to expand the Layers section.
3
4
Select the Layers to the left check box.
5
Clear the Layers on bottom check box.
6
Click  Build All Objects.
Mesh Control Edges 1 (mce1)
1
In the Geometry toolbar, click  Virtual Operations and choose Mesh Control Edges.
2
On the object fin, select Boundary 4 only.
3
In the Geometry toolbar, click  Build All.
Import a file that contains variables to be used in the model.
Definitions
Variables 1
1
In the Model Builder window, under Component 1 (comp1) right-click Definitions and choose Variables.
2
In the Settings window for Variables, locate the Variables section.
3
Click  Load from File.
4
Define the ionization Townsend coefficient using an analytic function.
Townsend coefficient
1
In the Home toolbar, click  Functions and choose Local>Analytic.
2
In the Settings window for Analytic, type Townsend coefficient in the Label text field.
3
In the Function name text field, type alpha.
4
Locate the Definition section. In the Expression text field, type 5.7*760*exp(-260*760/x).
5
Locate the Units section. In the table, enter the following settings:
6
In the Function text field, type cm^-1.
7
Locate the Plot Parameters section. In the table, enter the following settings:
Select to use the Local Field Approximation. This means that the electron mean energy equation is not solved.
Select to use Finite element (quadratic shape function). With this option streamline stabilization is automatically added.
Plasma (plas)
1
In the Model Builder window, under Component 1 (comp1) click Plasma (plas).
2
In the Settings window for Plasma, locate the Plasma Properties section.
3
From the Mean electron energy list, choose Local field approximation.
4
Click to expand the Discretization section. From the Formulation list, choose Finite element (quadratic shape function).
Create an electron impact ionization reaction that uses the Townsend coefficient previously defined.
Set the species M to be computed from mass constraint.
Set the species M+ to use initial condition from electronneutrality and set the ion mobility.
Electron Impact Reaction 1
1
In the Physics toolbar, click  Domains and choose Electron Impact Reaction.
2
In the Settings window for Electron Impact Reaction, locate the Reaction Formula section.
3
In the Formula text field, type e+M=>e+e+M+.
4
Locate the Collision Type section. From the Collision type list, choose Ionization.
5
In the Δε text field, type 10.
6
Locate the Reaction Parameters section. In the kf text field, type Ri.
Species: M
1
In the Model Builder window, click Species: M.
2
In the Settings window for Species, locate the Species Formula section.
3
Select the From mass constraint check box.
4
Locate the General Parameters section. From the Preset species data list, choose N2.
Species: M+
1
In the Model Builder window, click Species: M+.
2
In the Settings window for Species, locate the Species Formula section.
3
Select the Initial value from electroneutrality constraint check box.
4
Locate the General Parameters section. From the Preset species data list, choose N2.
5
Locate the Mobility and Diffusivity Expressions section. From the Specification list, choose Specify mobility, compute diffusivity.
6
Locate the Mobility Specification section. In the um text field, type mui.
Set electron mobility and diffusivity.
Plasma Model 1
1
In the Model Builder window, click Plasma Model 1.
2
In the Settings window for Plasma Model, locate the Electron Density and Energy section.
3
In the μe text field, type mue.
4
From the Electron transport properties list, choose Specify all.
5
6
In the De table, enter the following settings:
Set the initial conditions to use a profile defined in the variables.
Initial Values 1
1
In the Model Builder window, click Initial Values 1.
2
In the Settings window for Initial Values, locate the Initial Values section.
3
In the ne,0 text field, type ne0.
Apply a ground and a voltage to the bottom and top electrodes
The interaction of the streamer with the surface is not going to be modeled here. That is why Wall and Surface Reaction features, that define flux boundary conditions for electrons and ions, are not applied at the electrodes.
A fixed electron density is applied at the electrodes for stability reasons.
Ground 1
1
In the Physics toolbar, click  Boundaries and choose Ground.
2
Metal Contact 1
1
In the Physics toolbar, click  Boundaries and choose Metal Contact.
2
In the Settings window for Metal Contact, locate the Terminal section.
3
In the V0 text field, type V0.
4
Electron Density and Energy 1
1
In the Physics toolbar, click  Boundaries and choose Electron Density and Energy.
2
3
In the Settings window for Electron Density and Energy, locate the Electron Density and Energy section.
4
Select the Fix electron density check box.
5
In the new text field, type ne0_min.
Define a mesh that is very refined in the axis of symmetry where the streamer is going to propagate, and is coarse everywhere else.
Mesh 1
1
In the Model Builder window, under Component 1 (comp1) click Mesh 1.
2
In the Settings window for Mesh, locate the Sequence Type section.
3
From the list, choose User-controlled mesh.
Size
1
In the Model Builder window, under Component 1 (comp1)>Mesh 1 click Size.
2
In the Settings window for Size, locate the Element Size section.
3
From the Calibrate for list, choose General physics.
4
From the Predefined list, choose Normal.
Mapped 1
1
In the Mesh toolbar, click  Mapped.
2
Right-click Mapped 1 and choose Move Up.
3
In the Settings window for Mapped, locate the Domain Selection section.
4
From the Geometric entity level list, choose Domain.
5
6
Click to expand the Control Entities section. Clear the Smooth across removed control entities check box.
7
Click to expand the Reduce Element Skewness section.
Distribution 1
1
Right-click Mapped 1 and choose Distribution.
2
3
In the Settings window for Distribution, locate the Distribution section.
4
From the Distribution type list, choose Predefined.
5
In the Number of elements text field, type 30.
6
In the Element ratio text field, type 5.
7
From the Growth rate list, choose Exponential.
Distribution 2
1
In the Model Builder window, right-click Mapped 1 and choose Distribution.
2
3
In the Settings window for Distribution, locate the Distribution section.
4
In the Number of elements text field, type 600.
Free Triangular 1
1
In the Model Builder window, under Component 1 (comp1)>Mesh 1 click Free Triangular 1.
2
In the Settings window for Free Triangular, click to expand the Control Entities section.
3
Clear the Smooth across removed control entities check box.
4
Click  Build All.
Create a View that defines the aspect ratio used in the paper from where this example is based.
Definitions
View 2
1
In the Model Builder window, under Component 1 (comp1) right-click Definitions and choose View.
2
In the Settings window for View, locate the View section.
3
Select the Lock axis check box.
Axis
1
In the Model Builder window, expand the View 2 node, then click Axis.
2
In the Settings window for Axis, locate the Axis section.
3
In the r minimum text field, type -0.06.
4
In the r maximum text field, type 0.06.
5
In the z minimum text field, type 0.
6
In the z maximum text field, type 1.
7
From the View scale list, choose Manual.
8
In the y scale text field, type 0.17.
9
Click  Update.
All plots are going to be created manually. Also, create a mirror data set to have a better view of the streamer.
Study 1
1
In the Model Builder window, click Study 1.
2
In the Settings window for Study, locate the Study Settings section.
3
Clear the Generate default plots check box.
4
In the Study toolbar, click  Get Initial Value.
Results
In the Model Builder window, expand the Results node.
Mirror 2D 1
1
In the Model Builder window, expand the Results>Datasets node.
2
Right-click Results>Datasets and choose More 2D Datasets>Mirror 2D.
Electron Number Density
1
In the Results toolbar, click  2D Plot Group.
2
In the Settings window for 2D Plot Group, type Electron Number Density in the Label text field.
3
Locate the Data section. From the Dataset list, choose Mirror 2D 1.
4
Locate the Plot Settings section. From the View list, choose View 1.
Surface 1
1
Right-click Electron Number Density and choose Surface.
2
In the Settings window for Surface, locate the Expression section.
3
In the Expression text field, type plas.ne.
4
Click the  Zoom In button in the Graphics toolbar.
5
In the Electron Number Density toolbar, click  Plot.
Set the output times and choose to view the results while solving.
Study 1
Step 1: Time Dependent
1
In the Model Builder window, under Study 1 click Step 1: Time Dependent.
2
In the Settings window for Time Dependent, locate the Study Settings section.
3
From the Time unit list, choose ns.
4
In the Output times text field, type range(0,0.5,2.5).
5
Click to expand the Results While Solving section. Select the Plot check box.
6
From the Update at list, choose Time steps taken by solver.
7
In the Home toolbar, click  Compute.
Create more plots to show the electric potential, space charge density, and electric fields.
Start by creating a plot of the space charge density with superimposed electric potential contour lines.
Results
Electric Potential and Space Charge Density
1
In the Home toolbar, click  Add Plot Group and choose 2D Plot Group.
2
In the Settings window for 2D Plot Group, type Electric Potential and Space Charge Density in the Label text field.
3
Locate the Data section. From the Dataset list, choose Mirror 2D 1.
4
Locate the Plot Settings section. From the View list, choose View 1.
Surface 1
1
Right-click Electric Potential and Space Charge Density and choose Surface.
2
In the Settings window for Surface, locate the Expression section.
3
In the Expression text field, type plas.scharge.
4
In the Electric Potential and Space Charge Density toolbar, click  Plot.
Contour 1
1
In the Model Builder window, right-click Electric Potential and Space Charge Density and choose Contour.
2
In the Settings window for Contour, locate the Expression section.
3
In the Expression text field, type V.
4
Click the  Zoom In button in the Graphics toolbar.
5
In the Electric Potential and Space Charge Density toolbar, click  Plot.
Create an electron density contour plot to be compared with the figure from the reference paper.
Electron Density Contour
1
In the Home toolbar, click  Add Plot Group and choose 2D Plot Group.
2
In the Settings window for 2D Plot Group, type Electron Density Contour in the Label text field.
3
Locate the Data section. From the Dataset list, choose Mirror 2D 1.
Contour 1
1
Right-click Electron Density Contour and choose Contour.
2
In the Settings window for Contour, locate the Expression section.
3
In the Expression text field, type plas.ne.
4
Locate the Levels section. From the Entry method list, choose Levels.
5
In the Levels text field, type range(1.0e19,1.0e19,1.3e20).
6
In the Electron Density Contour toolbar, click  Plot.
Electron Density Contour
1
In the Model Builder window, click Electron Density Contour.
2
In the Settings window for 2D Plot Group, locate the Plot Settings section.
3
From the View list, choose View 2.
4
In the Electron Density Contour toolbar, click  Plot.
Create a 1D plot of the charged species number densities along the axis of symmetry.
Charged species number density
1
In the Home toolbar, click  Add Plot Group and choose 1D Plot Group.
2
In the Settings window for 1D Plot Group, type Charged species number density in the Label text field.
3
Click to expand the Title section. From the Title type list, choose None.
4
Locate the Plot Settings section. Select the y-axis label check box.
5
In the associated text field, type Number Density (1/m<sup>3</sup>).
Line Graph 1
1
Right-click Charged species number density and choose Line Graph.
2
In the Settings window for Line Graph, locate the y-Axis Data section.
3
In the Expression text field, type plas.ne.
4
5
Locate the x-Axis Data section. From the Parameter list, choose Expression.
6
In the Expression text field, type z.
7
Click to expand the Legends section. Select the Show legends check box.
8
Click to expand the Quality section. From the Resolution list, choose No refinement.
9
In the Charged species number density toolbar, click  Plot.
Line Graph 2
1
Right-click Line Graph 1 and choose Duplicate.
2
In the Settings window for Line Graph, locate the Legends section.
3
Clear the Show legends check box.
4
Locate the y-Axis Data section. In the Expression text field, type plas.n_wM_1p.
5
Click to expand the Coloring and Style section. Find the Line style subsection. From the Line list, choose Dotted.
6
From the Color list, choose Black.
Create a 1D plot of the z component of the electric field along the axis of symmetry.
Electric field
1
In the Home toolbar, click  Add Plot Group and choose 1D Plot Group.
2
In the Settings window for 1D Plot Group, type Electric field in the Label text field.
3
Locate the Title section. From the Title type list, choose None.
4
Locate the Axis section. Select the Manual axis limits check box.
5
In the x minimum text field, type 0.
6
In the y minimum text field, type -2e7.
7
In the y maximum text field, type 0.
8
Locate the Legend section. From the Position list, choose Lower right.
Line Graph 1
1
Right-click Electric field and choose Line Graph.
2
3
In the Settings window for Line Graph, locate the y-Axis Data section.
4
In the Expression text field, type plas.Ez.
5
Locate the x-Axis Data section. From the Parameter list, choose Expression.
6
In the Expression text field, type z.
7
Locate the Legends section. Select the Show legends check box.
8
In the Electric field toolbar, click  Plot.